Scott was ment to be the opposite to Cumbatch's portrayal of Sherlock, but that led to an idiotic, over acted, and less threatening than the Moriarty in The Great Mouse Detective.
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#3
Suggested by
Freemantle_uk
George Zucco - The Adventures of Sherlock Holmes
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#4
Suggested by
Phillip Hudson
Daniel Davis-Ship in a Bottle (Star Trek: The Next Generation)